Aminomethylenemalonates and Their Use in Heterocyclic by Alan R. Katritzky (Eds.)

By Alan R. Katritzky (Eds.)

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Io3 Marshall, J. A. , 1 Org. , 59, 7833 (1994). , 1 Chem. ,Chem. , 1995, 1273. lo' Menendez, E.. , and Gotor, V, 1 Chem. Soc.. Chem. , 1995, 989. , Cirillo, I? , and Panek, J. , 36, 8727 (1995). lo' Bodnar, P. , Palmer, W. , Shaw, J. , Smitrovich, J. , Sonnenberg, J. , Presley, A. , and Woerpel, K. A,, 1 Am. Chem. ,117, 10575 (1995). 'Ox Miura, T. , J Chem. , Perkin Trans. I , 1995, 2155. , Paschal, J. , and Loncharich, R. , 1 Org. , 60, 156 (1995). 110 Agganval, V. , Evans, G. , Thomas, A,, Mahon, M.

S), 1995, 394. , and Capriati, V, 1 Org. , 60, 2279 (1995). Willoughby, C. A. and Buchwald, S. , 1 Am. Chem. , 116, 11703 (1994). Prabhu, D. V and Laxmeshwar, N. , Asian 1 Chem. , 7, 278 (1995); Chem. , 122, 290125 (1995). , Dash, I? , Mishra, B. , and Behera, G. , 34A, 278 (1995); Chem. , 122, 313950 (1995). , Dash, P. , Mishra, B. , and Behera, G . , 34A, 227 (1995); Chem. , 123, 111340 (1995). , THEOCHEM, 334, 81 (1995); Chem. , 123, 55135 (1995). Eldin, S . , 1 Am. Chem. , 117, 4851 (1995).

ReEerences . . . . . . . . . . . . . . . . . . . . . . . y 1995 . Edited by A . C . Knipe and W. E . e. @A = 0) of the leaving-group phenolates and the nucleophile in the gas phase, particularly for the m-nitro compound. The low stability of T- in solution and stabilization by solvation of the transition state for the breakdown step result in all three formates reacting by a concerted mechanism. -OR I OH __ (2) R = Et, Pr' Scmm 2 OH I 4-MeC6H4-C-OR I 0- 2 Reactions of Acids and their Derivatives 37 0 SS II EtO-C-SAr (7) II EtO-C-SAr I+ -NH- (8) zwitterionic tetrahedral intermediate (3), with its breakdown rate-determining, is taking place as the crucial step.

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