By Alan R. Katritzky (Eds.)
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ReEerences . . . . . . . . . . . . . . . . . . . . . . . y 1995 . Edited by A . C . Knipe and W. E . e. @A = 0) of the leaving-group phenolates and the nucleophile in the gas phase, particularly for the m-nitro compound. The low stability of T- in solution and stabilization by solvation of the transition state for the breakdown step result in all three formates reacting by a concerted mechanism. -OR I OH __ (2) R = Et, Pr' Scmm 2 OH I 4-MeC6H4-C-OR I 0- 2 Reactions of Acids and their Derivatives 37 0 SS II EtO-C-SAr (7) II EtO-C-SAr I+ -NH- (8) zwitterionic tetrahedral intermediate (3), with its breakdown rate-determining, is taking place as the crucial step.