By Ilya Prigogine, Stuart A. Rice
Info at the evolution of dimension results in chemical dynamics is supplied through this publication. insurance contains structural versions for clusters produced in a unfastened jet growth, solid-liquid section behaviour in microclusters, the quantum mechanics of clusters, small cluster-reactions of van der Waals molecules, molecular floor chemistry, reactions of fuel ph ase steel clusters, vibrational rest in condensed stages and activated fee approaches in condensed stages.
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Extra resources for Advances in Chemical Physics, Vol.70 Part 2, Evolution of Size Effects in Chemical Dynamics (Wiley 1988)
25) shows the e v o l u t i o over a longer p e r i o d . A pur produced a peak of methane as shown (250°C). This i n c r e a s e i n CH^ production r a t e shows that H must be adsorbed (probably d i s s o c i ated as H) i n order to r e a c t , and a l s o that the s t e a d y - s t a t e s u r face must be l a r g e l y covered w i t h carbonaceous intermediate. Methane production seems t o be governed by the equation r = k C(a) H(a), w i t h C(a) > H(a) so that an i n c r e a s e i n H(a) leads t o a higher r a t e .
1979. 87, 501. Johnson, S. , an and desorption of CO and H 2 and surface reactions of alcohols by sulfur on Ni (100). ACS Symp. Ser. 1981; Madix, R. J. Adv. in Catal. 1980. 29. , and Fthenakis, V. Multiple isotope tracing of methanation over nickel catalyst. J. Catal. 1980. 65, 59. , Walter, Ε . , Zoulalian, A. and Gelas, M. A new operating method for the kinetic study of open systems by means of tracer elements. Chem. Eng. Sci. 1977. 32, 733. Happel, J. Transient tracing. Chem. Eng. Sci. 1978.
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