Advances in Chemical Physics, Vol.70 Part 2, Evolution of by Ilya Prigogine, Stuart A. Rice

By Ilya Prigogine, Stuart A. Rice

Info at the evolution of dimension results in chemical dynamics is supplied through this publication. insurance contains structural versions for clusters produced in a unfastened jet growth, solid-liquid section behaviour in microclusters, the quantum mechanics of clusters, small cluster-reactions of van der Waals molecules, molecular floor chemistry, reactions of fuel ph ase steel clusters, vibrational rest in condensed stages and activated fee approaches in condensed stages.

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25) shows the e v o l u t i o over a longer p e r i o d . A pur produced a peak of methane as shown (250°C). This i n c r e a s e i n CH^ production r a t e shows that H must be adsorbed (probably d i s s o c i ­ ated as H) i n order to r e a c t , and a l s o that the s t e a d y - s t a t e s u r ­ face must be l a r g e l y covered w i t h carbonaceous intermediate. Methane production seems t o be governed by the equation r = k C(a) H(a), w i t h C(a) > H(a) so that an i n c r e a s e i n H(a) leads t o a higher r a t e .

1979. 87, 501. Johnson, S. , an and desorption of CO and H 2 and surface reactions of alcohols by sulfur on Ni (100). ACS Symp. Ser. 1981; Madix, R. J. Adv. in Catal. 1980. 29. , and Fthenakis, V. Multiple isotope tracing of methanation over nickel catalyst. J. Catal. 1980. 65, 59. , Walter, Ε . , Zoulalian, A. and Gelas, M. A new operating method for the kinetic study of open systems by means of tracer elements. Chem. Eng. Sci. 1977. 32, 733. Happel, J. Transient tracing. Chem. Eng. Sci. 1978.

Catalysis 1977, 48, 262. Taylor, J. ; Weinberg, W. H. Surface S c i . 1978, 78, 259. ; Schmidt, L . D. Surface S c i . 1978, 76, 559. Close, J. ; White, J. M. J. Catalysis 1975, 36, 185. Campbell, C. ; Foyt, D. ; White, J. M. J. Phys. Chem. 1977, 81, 491. a. ; L a t t a , Ε. E . Surface S c i . 1977, 65, 245. b. ; Merrill, R. P. Surface S c i . 1976, 55, 227. c. McCabe, R. ; Schmidt, L . D. Surface S c i . 1976, 85, 60. Campbell, C. T . ; S h i , S. K . ; White, J. M. Appl. of Surface S c i . 1979, 2, 382.

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